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10.1038%2Fnmat2732
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methods summary
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Alginates (FMC Biopolymer) and agarose were covalently coupled with the integrin binding peptide (Gly)4-Arg-Gly-Asp-Ala-Ser-Ser-Lys-Tyr (Peptides International)>>17<<,20. PEGDM polymers were photo-crosslinked in the presence of acryloyl-PEG-GRGDS21.
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Alginates (FMC Biopolymer) and agarose were covalently coupled with the integrin binding peptide (Gly)4-Arg-Gly-Asp-Ala-Ser-Ser-Lys-Tyr (Peptides International)17,>>20<<. PEGDM polymers were photo-crosslinked in the presence of acryloyl-PEG-GRGDS21.
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PEGDM polymers were photo-crosslinked in the presence of acryloyl-PEG-GRGDS>>21<<. For cell encapsulation studies, mixtures of varying wt % polymer were mixed with stem cells (20 million clonally derived mMSC (D1) per mL, or 15 million hMSC/mL) and crosslinked to form hydrogels.
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FRET analysis of integrin-adhesion ligand bonds was performed by monitoring energy transfer between a membrane-intercalating fluorescein dye and rhodamine labeled peptides as previously described by Kong et al>>41<<. Clonally derived mMSC (D1) were labeled with 5-hexadecanoylaminofluorescein (Invitrogen) for 24 hr, and encapsulated into alginate matrices presenting G4RGDASSK(tetramethylrhodamine)Y-OH.
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DFRET was used to calculate the number of integrin-RGD bonds based on a linear calibration curve generated by performing parallel FRET-binding and 125I-RGD binding studies in solution>>41<<.
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